瞿赞(Qu Zan)
研究员
电子邮件:quzan@sjtu.edu.cn
办公室电话:02154745591
办公地点:上海交通大学闵行校区环境科学楼1031室
团队网页:http://air.sjtu.edu.cn/
研究方向
- 大气污染控制技术
- 重金属控制技术
- 便携式烟气净化工艺与装备
个人简历
1995.09-1999.07,毕业于郑州大学化工学院,获得学士学位;
1999.09-2002.07,毕业于郑州大学化工学院,获得硕士学位;
2003.03-2007.04,毕业于bwin必赢,获得博士学位;
2007.04-2008.03, 美国加州大学劳伦斯-伯克利国家实验室,博士后;
2008.03-2011.12, bwin必赢,讲师;
2012.01-2016.12, bwin必赢,副教授;
2015.09-2016.09, 美国佐治亚理工学院,访问学者;
2017.01-至今,bwin必赢,研究员。
研究论文
- Qu, Z.; Yan, N.Q.*; Zhao, Y.F.; Jia, J.P.; Wu, D. Removal of dibenzothiophene from the simulated petroleum by gamma-irradation induced reaction. Energy Fuels, 2006, 20, 142-147.
- Qu, Z.; Yan, N.Q.*; Jia, J.P.; Wu, D. Removal of dibenzothiophene from simulated petroleum by integrated gamma-irradiation and Zr/alumina catalyst. Applied Catalysis B: Environmental. 2007, 71, 108-115.
- Qu, Z.; Yan N.Q.*; Liu, P.; Chi, Y.; Jia, J.P. Bromine chloride as an oxidant to improve elemental mercury removal from coal-fired flue gas. Environmental Science Technology. 2009, 43, 8610-8615.
- Qu, Z.; Chang, J.J.; Hsiung, T.L.; Yan, N.Q.; Wang, H.P.; Dod, R.; Chang, S.G.*; Miller, C. Halides on Carbonaceous Materials for Enhanced Capture of Hg0: Mechanistic Study. Energy Fuels. 2010, 24, 3534-3539.
- Qu, Z.; Yan, N.Q.*; Liu, P.; Jia, J.P.; Yang, S.J. The role of iodine monochloride for the oxidation of elemental mercury. Journal of Hazardous Materials. 2010, 183(1-3), 132-137.
- Qu, Z.; Yan N.Q.*; Liu, P.; Guo, Y.F.; Jia, J.P. Oxidation and stabilization of elemental mercury from coal-fired flue gas by sulfur monobromide. Environmental Science Technology. 2010, 44, 3889-3894.
- Yan, N.Q.*; Chen, W.M.; Chen, J.; Qu, Z.*; Guo, Y.F.; Yang, S.J.; Jia, J.P. Significance of RuO2 Modified SCR catalyst for elemental mercury oxidation in coal-fired flue gas. Environmental Science Technology. 2011, 45, 5725-5730.
- Xie, J.K.; Qu, Z.*; Yan, N.Q.*; Yang, S.J.; Chen, W.M.; Hu, L.G.; Huang, W.J.; Liu, P. Novel regenerable sorbent based on Zr–Mn binary metal oxides for flue gas mercury retention and recovery. Journal of Hazardous Materials. 2013, 261, 206-213.
- Xie, J.K.; Xu, H.M.; Qu, Z.*; Huang, W.J.; Chen, W.M.; Ma, Y.P.; Zhao, S.J.; Liu, P.; Yan, N.Q.* Sn–Mn binary metal oxides as non-carbon sorbent for mercury removal in a wide-temperature window. Journal of Colloid and Interface Science. 2014, 428, 121-127.
- Chen, W.M.; Ma, Y.P.; Yan, N.Q.*; Qu, Z.*; Yang, S.J.; Xie, J.K.; Guo, Y.F.; Hu, L.G.; Jia, J.P. The co-benefit of elemental mercury oxidation and slip ammonia abatement with SCR-Plus catalysts. Fuel. 2014, 133, 263-269.
- Ma, Y.P.; Xu, H.M.; Qu, Z.*; Yan, N.Q.*; Wang, W.H. Absorption characteristics of elemental mercury in mercury chloride solutions. Journal of Environmental Sciences. 2014, 2257-2265.
- Chen, W.M.; Ma, Y.P.; Qu, Z.*; Liu, Q.H.; Huang, W.J.; Hu, X.F.; Yan, N.Q.* Mechanism of the Selective Catalytic Oxidation of Slip Ammonia over Ru-Modified Ce−Zr Complexes Determined by in Situ Diffuse Reflectance Infrared Fourier Transform Spectroscopy. Environmental Science Technology. 2014, 48, 12199-12205.
- Ma, Y.P.; Qu, Z.*; Xu, H.M.; Wang, W.H.; Yan, N.Q. Investigation on mercury removal method from flue gas in the presence of sulfur dioxide. Journal of Hazardous Materials. 2014, 279, 289-295.
- Qu, Z.; Yan, L.L.; Li, L.*; Xu, J.F.; Liu, M.M.; Li, Z.C.; Yan, N.Q.* Ultraeffective ZnS nanocrystals sorbent for mercury (II) removal based on size-dependent cation exchange. ACS Applied Materials Interfaces. 2014, 6, 18026-18032.
- Xu, H.M.; Xie, J.K.; Ma, Y.P.; Qu, Z.*; Zhao, S.J.; Chen, W.M.; Huang, W.J.; Yan, N.Q.* The cooperation of Fe-Sn in a MnOx complex sorbent used for capturing elemental mercury. Fuel. 2015, 140, 803-809.
- Zhao, S.J.; Qu, Z.*; Yan, N.Q.*; Li, Z.; Zhu, W.F.; Pan, J.; Xu, J.F.; Li, M.D. Ag-modified AgI-TiO2 as an excellent and durable catalyst for catalytic oxidation of elemental mercury. RSC Advances. 2015, 5, 30841-30850.
- Xu, H.M.; Qu, Z.*; Huang, W.J.; Mei, J.; Chen, W.M.; Zhao, S.J.; Yan, N.Q. Regenerable Ag/graphene sorbent for elemental mercury capture at ambient temperature. Colloids and Surfaces A: Physicochemical and Engineering Aspects. 2015, 476, 83-89.
- Ma, Y.P.; Xu, H.M.; Qu, Z.*; Yan, N.Q.; Wang, W.H. Removal of mercury from flue gas from nonferrous metal smelting, by use of mercury chloride solution, and mechanisms of inhibition by sulfur dioxide. Research on Chemical Intermediates. 2015, 41, 5889-5905.
- Xu, H.M.; Qu, Z.*; Zong, C.X.; Huang, W.J.; Quan, F.Q.; Yan, N.Q.* MnOx/graphene for the catalytic oxidation and adsorption of elemental mercury. Environmental Science Technology. 2015, 49, 6823-6830.
- Qu, Z.; Xie, J.K.; Xu, H.M.; Chen, W.M.; Yan, N.Q.* Regenerable sorbent with a high capacity for elemental mercury removal and recycling from the simulated flue gas at a low temperature. Energy Fuels. 2015, 29(10), 6187-6196.
- Huang, W.J.; Xu, H.M.; Qu, Z.*; Zhao, S.J.; Chen, W.M.; Yan, N.Q.* Significance of Fe2O3 modifed SCR catalyst for gas-phase elemental mercury oxidation in coal-fired flue gas. Fuel Processing Technology. 2016, 149, 23-28.
- Huang, W.J.; Qu, Z.*; Chen, W.M.; Xu, H.M.; Yan, N.Q.* An enhancement method for the elemental mercury removal from coal-fired flue gas based on novel discharge activation reactor. Fuel. 2016, 171, 59-64.
- Xu, J.F.; Qu, Z.*; Yan, N.Q.; Zhao, Y.X.; Hu, X.F.; Li, L.* Size-dependent nanocrystal sorbent for copper removal from water. Chemical Engineering Journal. 2016, 284, 565-570.
- Zhu, Z.X.; Ma, Y.P.; Qu, Z.*; Fang, L.; Zhang, W.Y.; Yan, N.Q. Study on a new wet flue gas desulfurization method based on the Bunsen reaction of sulfur-iodine thermochemical cycle. Fuel. 2017, 195, 33-37.
- Qu, Z.*; Fang, L.; Chen, D.Y.; Xu, H.M.; Yan, N.Q. Effective and regenerable Ag/graphene adsorbent for Hg(II) removal from aqueous solution. Fuel. 2017, 203, 128-134.
- Chen, D.Y.; Zhao, S.J.*; Qu, Z.*; Yan, N.Q. Cu-BTC as a novel material for elemental mercury removal from sintering gas. Fuel. 2018, 217, 297-305.
- Fang, L.; Li, L.; Qu, Z.*; Xu, H.M.; Xu, J. F.; Yan, N.Q. A novel method for the sequential removal and separation of multiple heavy metals from wastewater. Journal of Hazardous Materials. 2018, 342, 617-624.
- Quan, Z.W.; Huang, W.J.; Liao, Y.; Liu, W.; Xu, H.M.; Yan, N.Q.; Qu, Z.* Study on the regenerable sulfur-resistant sorbent for mercury removal from nonferrous metal smelting flue gas. Fuel. 2019, 241, 451-458.
- Liao, Y.; Xu, H.M.; Liu, W.; Ni, H.F.; Zhang, X.G.; Zhai, A.P.; Quan, Z.W.; Qu, Z.*; Yan, N.Q. One step interface activation of ZnS using cupric ions for mercury recovery from nonferrous smelting flue gas. Environmental Science Technology. 2019, 53, 4511-4518.
- Liu, W.; Zhou, Y.X.; Hua, Y.F.; Peng, B.; Deng, M.; Yan, N.Q.; Qu, Z.* A Sulfur-resistant CuS-modified active coke for mercury removal from solid waste incineration flue gas. Environmental Science and Pollution Research. 2019, 26, 24831-24839.
- Li, J.X.; Xu, H.M.; Liao, Y.; Qiu, Y.X.; Yan, N.Q.; Qu, Z.* Atomically Dispersed Manganese on a Carbon-Based Material for the Capture of Gaseous Mercury: Mechanisms and Environmental Applications. Environmental Science Technology. 2020, 54(8), 5249-5257.
- Wang, L.L.; Xu, H.M.; Qiu, Y.X.; Liu, X.S.; Huang, W.J.; Yan, N.Q.; Qu, Z.* Utilization of Ag nanoparticles anchored in covalent organic frameworks for mercury removal from acidic waste water. Journal of Hazardous Materials. 2020, 389, 121824.
- Liu, W.; Xu, H.M.; Liao, Y.; Wang, Y.L.; Yan, N.Q.; Qu, Z.* Co-doped ZnS with large adsorption capacity for recovering Hg0 from non-ferrous metal smelting gas as a co-benefit of electrostatic demisters. Environmental Science and Pollution Reserach. 2020, 27, 20469–20477.
- Mei, J.; Liao, Y.; Qin, R.Y.; Sun, P.X.; Wang, C.; Ma, Y.P.; Qu, Z.*; Yan, N.Q.; Yang, S.J.* Acceleration of Hg0 adsorption onto natural sphalerite by Cu2+ activation during flotation: mechanism and applications in Hg0 recovery. Environmental Science Technology. 2020, 54, 7687-7696.
- Liao, Y.; Liu, W.; Xu, H.M.; Hong, Q.Y.; Wang, Y.L.; Qu, Z.*; Yan, N.Q. Zinc concentration internal circulation technology for elemental mercury recovery from zinc smelting flue gas. Fuel. 2020, 280, 118566.
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Wang, L.L.; Deng, M.; Xu, H.M.; Li, W.W.; Huang, W.J.; Yan, N.Q.; Zhou, Y.X.; Chen, J.S.; Qu, Z.* Selective reductive removal of silver ions from acidic solutions by redox-active covalent organic frameworks. ACS Applied Materials & Interfaces. 2020, 12, 37619-37627.
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Sun, Y.N.; Deng, M.; Huang, W.J.; Zhou, Y.X.; Zhao, Y.; Chen, J.S.; Yan, N.Q.; Qu, Z.* Radical-Induced Oxidation Removal of Mercury by Ozone Coupled with Bromine. ACS ES&T Engineering. 2021, 1, 110-116.
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Sun, Y.N.; Xie, J.K.; Huang, W.J.; Li, G.; Li, S.C.; Cui, P.; Xu, H.M.; Qu, Z.*; Yan, N.Q. Novel product-adjustable technology using Wellman-Lord method coupled with sodium-alkali for SO2 removal and regeneration from smelting gas. Fuel. 2021, 288, 119714.
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Wang, L.L.; Zhang, K.; Luo, J.M.; Ma, J.Y.; Ji, W.X.; Hong, Q.Y.; Xu, H.M.; Huang, W.J.; Yan, N.Q.; Qu, Z.* Metastable Facet-Controlled Cu2WS4 Single Crystals with Enhanced Adsorption Activity for Gaseous Elemental Mercury. Environmental Science Technology. 2021, 55, 5347-5356.
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Li, J.X.; Xu, H.M.; Huang, Z.J.; Hong, Q.Y.; Qiu, Y.X.; Yan, N.Q.; Qu, Z.* Strengthen the affinity of element mercury on the carbon-based material by adjusting the coordination environment of single-site manganese. Environmental Science Technology. 2021, 55, 14126−14135.
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Xu, H.M.; Hong, Q.Y.; Li, J.X.; Liao, Y.; Huang, W.J.; Qu, Z.*; Yan, N.Q. Heterogeneous Reaction Mechanisms and Functional Materials for Elemental Mercury Removal from Industrial Flue Gas. ACS ES&T Engineering. 2021, 1, 10, 1383–1400.
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Wang, L.L.; Ji, L.P.; Li, W.W.; Zhang, K.; Xu, H.M.; Huang, W.J.; Yan, N.Q.; Qu, Z.* Fabrication of Cu2S hollow nanocages with enhanced high-temperature adsorption activity and recyclability for elemental mercury capture. Chemical Engineering Journal. 2022, 427, 130935.
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Huang, W.J.; Xu, H.M.; Liu, X.S.; Wang, L.L.; Li, S.T.; Ji, L.P.; Qu, Z.*; Yan, N.Q. Surface protection method for the magnetic core using covalent organic framework shells and its application in As(III) depth removal from acid wastewater. Journal of Environmental Sciences, 2022, 115, 1-9.
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Li, W.W.; Gao, G.Q.; Wang, L.L.; Xu, H.M.; Huang, W.J.; Yan, N.Q.; Qu, Z.* Dual confinement strategy based on metal-organic frameworks to synthesize MnOx@ZrO2 catalysts for toluene catalytic oxidation. Fuel, 2022, 320, 123983.
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Gao, G.Q.; Liao, Y.; Li, W.W.; Li, Z.H.; Xu, H.M.; Huang, W.J.; Yan, N.Q.; Qu, Z.* Active Surface RuOx Species Originating from Size-Driving Self-Dispersion Process for Toluene Catalytic Combustion. Chemical Engineering Journal, 2022, 441, 136127.
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Wang, L.L.; Zhang, K.; Li, J.X.; Shen, X.R.; Yan, N.Q.; Zhao, H.Z.; Qu, Z.* Engineering of Defect-Rich Cu2WS4 Nano-homojunctions Anchored on Covalent Organic Frameworks for Enhanced Gaseous Elemental Mercury Removal. Environmental Science Technology. 2022, 56, 22, 16240-16248.
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Huang, W.J.; Zong, C.X.; Liu, Z.S.; Hong, Q.Y.; Ji, L.P.; Xu, H.M.; Qu, Z.*; Yan, N.Q. Cubic SAPO-34 supported MnOx for low-temperature gaseous mercury oxidation and adsorption from coal-fired flue gas. Fuel. 2023, 332, 126142.
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Li, W.W.; Liu, Z.S.; Wang, L.L.; Gao, G.Q.; Xu, H.M.; Huang, W.J.; Yan, N.Q.; Wang, H.W.; Qu, Z.* FeSx@MOF-808 composite for efficient As(III) removal from wastewater: behavior and mechanism. Journal of Hazardous Materials. 2023, 446, 130681.
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Li, J.X.; Li, H.L.; Xu, H.M.; Hong, Q.Y.; Ji, L.P.; Liu, Z.S.; Qiu, Y.X.; Huang, W.J.; Yan, N.Q.; Qu, Z.* Regulated adsorption sites using atomically single cluster over biochar for efficient elemental mercury uptake. Biochar. 2023, 5(13).
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Xu, H.M.; Hong, Q.Y.; Zhang, Z.Y.; Cai, X.L.; Fan, Y.R.; Liu, Z.S.; Huang, W.J.; Yan, N.Q.; Qu, Z.*; Zhang, L.Z.* SO2-Driven In Situ Formation of Superstable Hg3Se2Cl2 for Effective Flue Gas Mercury Removal. Environmental Science Technology. 2023, 57, 13, 5424-5432.
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Chen, C.; Huang, W.J.; Xu, H.M.; Liu, Z.S.; Li, X.W.; Shi, H.Z.; Yu, Y.M.; Qu Z.*; Yan, N.Q. CO2 sequestration and CaCO3 recovery with steel slag by a novel two-step leaching and carbonation method. Science of the Total Environment. 2023, 891, 164203.
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Gao, G.Q.; Liu, W.; Liu, Z.S.; Li, Z.H.; Xu, H.M.; Huang, W.J.; Yan, N.Q.; Qu, Z.* Electron Donation from Boron Suboxides via Strong p–d Orbital Hybridization Boosts Molecular O2 Activation on Ru/TiO2 for Low-Temperature Dibromomethane Oxidation. Environmental Science Technology. 2023, 57, 45, 17566–17576.
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Liu, Z.S.; Xu, H.M.; Fan, Y.R.; Hong, Q.Y.; Huang, W.J.; Yu, F.; Qu, Z.*; Yan, N.Q. Cation Concavities Induced d-Band Electronic Modulation on Co/FeOx Nanostructure to Activate Molecular and Interfacial Oxygen for CO Oxidation. Environmental Science Technology. 2023, 57, 50, 21272–21283
科研项目
一、国家自然科学基金委项目
1. 国家自然科学基金(青年基金),弱电离环境中卤硫化物对烟气零价汞的去除机制研究,50908145,课题负责人;
2. 国家自然科学基金(面上项目),含溴除汞促进剂在烟气除汞过程中的归趋及其次生污染控制研究,51278294,课题负责人;
3. 国家自然科学基金(面上项目),有色金属冶炼烟气汞定向形态调控回收技术原理研究,21677096,课题负责人;
4. 国家自然科学基金(面上项目),基于高温过滤/催化体系协同脱除焚烧烟气持久性有机污染物与汞的应用基础研究,52070129,课题负责人;
二、科技部项目
1. 国家高技术研究发展计划项目(863计划),燃煤锅炉烟气汞污染排放控制技术,2007AA06Z340,子课题负责人;
2. 国家高技术研究发展计划项目(863计划),工业锅炉湿法脱硫脱硝脱汞技术与示范,2011AA060801,子课题负责人;
3. 国家高技术研究发展计划项目(863计划),有色炉窑烟气高浓度SO2回收及重金属协同控制技术研究与示范, 2012AA062504,子课题负责人;
4. 国家重点基础研究发展计划项目(973计划),汞污染排放过程形态调控机制及控制技术原理,2013CB430005,子课题负责人;
5. 国家重点研发计划项目,有色金属冶炼烟气多污染物协同控制技术,2017YFC0210500,子课题负责人;
6. 国家重点研发计划项目,高原高寒地区灾害现场安置装备关键技术与装备研究及应用示范,2017YFC0806300,子课题负责人;
7. 生态环境部对外合作中心"中国履行《关于汞的水俣公约》能力建设项目",四川省有色金属冶炼行业含汞废物环境无害化管理现状评估,FECO/LY4/S/22/013,课题负责人。
荣获奖项
- 上海交通大学优秀共产党员,2011年;
- 上海交通大学“SMC-晨星青年学者”奖励计划(B类),2012年;
- 上海交通大学“晨星-优秀学者"奖励计划(教授A类),2018年;
- 《燃煤烟气汞及其它污染物协同控制技术研发与应用》,教育部技术发明二等奖,2018年;
- 《铁基尖晶石材料用于协同除汞脱硝的应用基础研究》,上海市自然科学二等奖,2018年;
- 《有色金属冶炼行业污酸处理及资源化利用关键技术》,河南省教育厅科技成果一等奖,2019年;
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《有色金属冶炼行业污酸处理及资源化利用关键技术》,河南省科技进步三等奖,2020年;
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《疫情医疗废物应急处置装置研发与应用》,中国发明协会发明创业成果一等奖,2020年;
- 上海交通大学优秀共产党员,2021年;
- 《我国汞污染特征、环境过程及减排技术原理》,贵州省自然科学一等奖,2021年。
- 《燃煤烟气硫-硝-汞联合脱除关键技术研究》,中华环保联合会科技进步二等奖,2022年。
- 《有色冶炼烟气多污染物协同控制耦合资源化技术与应用》(发明),中国有色金属工业科学技术一等奖,2022年。
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《有色金属冶炼烟气多污染物协同控制技术研发与应用》,教育部技术发明一等奖,2022年。
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《工业烟气超低排放与协同控制关键材料及技术装备》,浙江省科技进步一等奖,2023年。